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Anjali's filmography is a testament to her versatility as an actress. She has appeared in a wide range of films across multiple languages, including Tamil, Telugu, Malayalam, and Kannada. Some of her notable films include:

While she debuted in the 2006 Telugu thriller , her true breakthrough came with the critically acclaimed Tamil film Kattradhu Thamizh (2007). Her portrayal of Anandhi earned her the Filmfare Award for Best Female Debut, marking her as a "breath of fresh air" in the industry.

Unlike the glamorous heroines of her time, Anjali carved a niche for herself as a versatile character artist and a powerful leading lady. She is best known for her realistic acting, emotional depth, and willingness to take on rural and rustic roles. Her breakthrough came with the Telugu film Photo (2006), but it was her performance in the Tamil blockbuster Angaadi Theru (2010) that earned her the Tamil Nadu State Film Award for Best Actress.